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Systematic evaluation of one-dimensional-to-two-dimensional near-infrared spectroscopy transformations with deep learning for quantifying coconut sap adulteration
(2026-10-01)
Lapcharoensuk, Ravipat
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Sitorus, Agustami
Near-infrared (NIR) spectroscopy have limitations when combined with deep learning (DL) algorithms because they rely on low-dimensional datasets. Therefore, we investigated the potential of transforming one-dimensional (1D) NIR spectra into two-dimensional (2D) spectrograms using synchronous and asynchronous techniques and the continuous wavelet transform (CWT) and their effectiveness by integrating with DL for detecting adulteration in coconut sap. NIR spectra (12,500–4000 cm<sup>−1</sup>) were collected from binary mixtures (0%–100%; w /w). The performance of all DL (convolutional neural networks-CNN, AlexNet and ResNet) models was compared with that of partial least squares (PLS). The models were ranked in the mentioned order based on their performances: 2D-CWT ' 2D-asynchronous ' 2D-synchronous ' 1D/2D-PLS. The important features of the best model can be explained and visualized using gradient-weighted-class-activation-mapping. The findings highlight that the 1D-to-2D NIR data transformation combined with DL is a highly robust approach because it addresses the feature representation gap in NIR data and effectively captures the spatial–spectral correlations.
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Low-cost Multispectral Acquisition Device Coupled with Machine Learning for Detecting Adulteration of Honey
(2026-07-15)
Boodnon, Wutthiphong
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Lunvongsa, Thayanont
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Suntisakoonwong, Phanchay
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Sitorus, Agustami
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Lapcharoensuk, Ravipat
Honey is a natural sweetener created by honeybees from the nectar of flowers. Honey's extensive health benefits have led to its widespread use across multiple industries. Honey adulteration with inferior substances undermines its quality, reducing natural nutrients and antioxidants, and diminishing its health benefits. This study aimed to study the possibility of detection of honey adulteration with a low-cost multispectral device coupled with machine learning. The adulterated honey came from deliberate adulteration with cane syrup in the 1 to 90% range. Spectral data was collected for pure honey and the adulterated honey samples at the wavelengths of 610, 680, 730, 760, 810, and 860 nm. The detection models for distinguishing pure and adulterated honey were developed by Linear Discriminant Analysis (LDA), Partial Least Squares Discriminant Analysis (PLS-DA), C-Support Vector Machine (C-SVM), and K-Nearest Neighbors (KNN). All models achieved high accuracy between 0.91 and 0.98 and maintained balanced precision and recall metrics. This study serves as a guideline for developing a low-cost portable honey authentication device that is practical for real-world applications.
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NIR Spectroscopy for Non-Destructive Prediction of Greenhouse Gas Emissions and Global Warming Potential by Biomass Combustion
(2026-05-01)
Sirisomboon, Panmanas
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Gyawali, Prakash
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Posom, Jetsada
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Lapcharoensuk, Ravipat
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Shrestha, Bim Prasad
Greenhouse gas (GHG) emissions from biomass combustion include carbon dioxide (CO<inf>2</inf>), methane (CH<inf>4</inf>) and nitrous oxide (N<inf>2</inf>O), which cause climate change and global warming. By measuring GHG emissions by biomass combustion, a potent protocol for the calculation of global warming potential (GWP), which is how much the global temperature has risen due to combustion processes, can be achieved, contributing to determining the mean reduction in global temperature rise and fostering a transition towards more sustainable energy systems. Additionally, warning can be given of the GHG and GWP risks associated with different species of biomass. This review includes the GHG emissions and GWP of biomass combustion and their measurement and estimation directly through biomass sample combustion, using unmanned aerial vehicles (UAVs) and satellite measurements of radiation interacting with atmospheric gases, or satellite-derived data and calculations according to IPCC guidelines. In addition, the relationship of lignocellulosic compounds and elements in biomass to HHV and GHG emissions is described. The key mechanism of molecular vibration of hydrogen bonds in biomass caused by NIR radiation related to GHG emissions is revealed and recorded regarding the possibility of using NIR spectroscopy for the prediction of GHG emissions and GWP. Calculation examples for sugarcane bagasse and other biomass species are shown. The comparative advantages and limitations of NIR spectroscopy with respect to other methods are included. These factors lead to elucidation of the possibility of using NIR spectroscopy for non-destructive prediction of GHG emissions. In this review, the feasibility of using NIR spectroscopy to evaluate GHG emissions, GWP and emission factors (EFs) as an alternative to IPCC estimation methods related to climate change by biomass combustion is confirmed. NIR spectroscopy is a novel methodology for predicting GHG emissions and GWP directly from intact chip or powder biomass spectral data without explicit gas measurement. This article records the essential spectroscopic knowledge of biomass polymer valorization that is of value in polymer science.
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Interpretable ANN-Based Computer Vision System for Mangosteen Ripeness Detection for Export Markets
(2026-01-21)
Lapcharoensuk, Ravipat
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Tosribunjerd, Naphon
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Poonpakdee, Pasu
Mangosteen is a high-value tropical fruit widely consumed and exported from Thailand. Mangosteen ripeness classification is crucial for export quality control, but manual grading leads to inconsistency and inefficiency. This study presents a computer vision system using an Artificial neural network to classify mangosteen into ripe, semi-ripe, and unripe stages based on peel color. A dataset of 378 images was collected and processed to extract 40 color-based features across multiple color spaces. Principal Component Analysis demonstrated non-linear separability among the ripeness classes. SMOTE and Gaussian noise augmentation were used to tackle data imbalance and enhance generalizability. The model reached a 95% accuracy rate and displayed flawless precision and recall for the ripe class. Integrated Gradients analysis highlighted the importance of the red-green color component (CIELAB a*) in the classification process. The proposed method demonstrates a low-cost, interpretable, and efficient solution suitable for real-world application in the mangosteen export industry.
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Quantitative analysis based on image processing combined with machine learning and deep learning to determine the adulteration in nutmeg powder
(2025-10-01)
Sitorus, Agustami
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Pambudi, Suluh
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Boodnon, Wutthiphong
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Lapcharoensuk, Ravipat
The global demand for nutmeg powder has increased, raising the risk of adulteration and necessitating an efficient and cost-effective screening method. The objective of this study is to develop a calibration model to predict the adulteration of nutmeg powder by cinnamon powder using a novel approach by integrating image processing with machine learning (ML) and deep learning (DL). Eight regressors, including four ML regressors (multiple linear ridge regression–MLRR, partial least squares regression–PLSR, multi-layer perceptron–MLP, and adaptive boosting–ABS) and four DL regressors (convolutional neural networks–CNN, AlexNET, residual networks–ResNET, and GoogleNET), were employed to analyze 1800 images of adulteration samples ranging from 0 % to 35 % (w/w). Among ML models, MLP achieved the highest accuracy in prediction (R<inf>p</inf>²=0.922, RMSEP=2.804 %, RPD=3.59), while PLSR (R<inf>p</inf>²=0.876, RMSEP=3.538 %, RPD=2.84), MLRR (R<inf>p</inf>²=0.872, RMSEP=3.596 %, RPD=2.80), and ABS (R<inf>p</inf>²=0.849, RMSEP=3.904 %, RPD=2.58) underperformed. For DL, ResNET (R<inf>p</inf>²=0.882, RMSEP=3.416 %, RPD=2.91) surpassed CNN (R<inf>p</inf>²=0.876, RMSEP=3.505 %, RPD=2.84), AlexNET (R<inf>p</inf>²=0.801, RMSEP=4.429 %, RPD=2.24), and GoogleNET (R<inf>p</inf>²=0.751, RMSEP=4.963 %, RPD=2.00). The MLP's superiority highlights its compatibility with ORB-based feature extraction for nonlinear adulteration patterns, outperforming complex DL architectures. This research highlights the potential of image processing supported by ML and DL as a rapid and low-cost tool for future nutmeg powder adulteration screening.
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Revealing the Power of Deep Learning in Quality Assessment of Mango and Mangosteen Purée Using NIR Spectral Data
(2025-09-01)
Pornchaloempong, Pimpen
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Sharma, Sneha
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Phanomsophon, Thitima
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Sirisomboon, Panmanas
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Lapcharoensuk, Ravipat
The quality control of fruit purée products such as mango and mangosteen is crucial for maintaining consumer satisfaction and meeting industry standards. Traditional destructive techniques for assessing key quality parameters like the soluble solid content (SSC) and titratable acidity (TA) are labor-intensive and time-consuming; prompting the need for rapid, nondestructive alternatives. This study investigated the use of deep learning (DL) models including Simple-CNN, AlexNet, EfficientNetB0, MobileNetV2, and ResNeXt for predicting SSC and TA in mango and mangosteen purée and compared their performance with the conventional chemometric method partial least squares regression (PLSR). Spectral data were preprocessed and evaluated using 10-fold cross-validation. For mango purée, the Simple-CNN model achieved the highest predictive accuracy for both SSC (coefficient of determination of cross-validation ((Formula presented.)) = 0.914, root mean square error of cross-validation (RMSE<inf>CV</inf>) = 0.688, the ratio of prediction to deviation of cross-validation (RPD<inf>CV</inf>) = 3.367) and TA ((Formula presented.) = 0.762, RMSE<inf>CV</inf> = 0.037, RPD<inf>CV</inf> = 2.864), demonstrating a statistically significant improvement over PLSR. For the mangosteen purée, AlexNet exhibited the best SSC prediction performance ((Formula presented.) = 0.702, RMSE<inf>CV</inf> = 0.471, RPD<inf>CV</inf> = 1.666), though the RPD<inf>CV</inf> values (<2.0) indicated limited applicability for precise quantification. TA prediction in mangosteen purée showed low variance in the reference values (standard deviation (SD) = 0.048), which may have restricted model performance. These results highlight the potential of DL for improving NIR-based quality evaluation of fruit purée, while also pointing to the need for further refinement to ensure interpretability, robustness, and practical deployment in industrial quality control.
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Monitoring Pesticide Residue on Bok Choi using Convolution Neural Network with NIR spectral Data
(2024-12-29)
Lapcharoensuk, Ravipat
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Fhaykamta, Chawisa
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Anurak, Watcharaporn
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Chadwut, Wasita
Deep learning (DL) has been applied in agriculture, especially quality control in agricultural processing. One key area of interest is the detection and monitoring of pesticide residues in crops. The most popular measurement tool for nondestructive monitoring of pesticide residues is near-infrared spectroscopy (NIRS). A combination of CNN model with NIR spectral data was developed for monitoring pesticide residue on bok choi. The NIR spectral of bok choi with and without pesticide residue (chlorpyrifos) was collected in wavelength range between 908 and 1676 nm. A simple structure of CNN was modified for a one-dimensional task and this deep learning architecture was trained for classification of the bok choi samples. The results showed prefect prediction with 100% accuracy, precision, recall and specificity. This study also found that deep learning for NIR spectroscopy data requires less processing than traditional machine learning while still achieving great results.
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Development of automatic tuning for combined preprocessing and hyperparameters of machine learning and its application to NIR spectral data of coconut milk adulteration
(2024-11-01)
Sitorus, Agustami
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Lapcharoensuk, Ravipat
This study proposed a novel approach to automatically select the preprocessing methods and hyperparameters of machine learning (ML) algorithms based on their best performance in cross-validation for near-infrared (NIR) spectroscopy data. The proposed method simultaneously incorporates single or multiple-preprocessing steps and tunes hyperparameters to determine the best model performance for FT-NIR and Micro-NIR spectral data of coconut milk adulteration with distilled water and mature coconut water in the range of 0%–50%. Computational experiments were conducted using nine single preprocessing types, three types of ML classifier (linear discriminant analysis (LDA), k-nearest neighbour (KNN), multilayer perceptron (MLP)) and three types of ML regressor (partial least squares (PLS), KNN, MLP). The proposed performance strategy effectively addressed and produced satisfactory outcomes for classification and regression challenges in coconut milk adulteration. Finally, the results demonstrated that the proposed approach can more accurately determine the best model, particularly for NIR spectroscopy of coconut milk adulteration.
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Discrimination model of geographical area from coconut milk by near-infrared spectroscopy: Exploration in tandem with classical chemometrics, machine learning, and deep learning
(2024-11-01)
Sitorus, Agustami
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Lapcharoensuk, Ravipat
This work proposes exploring the discrimination model by near-infrared (NIR) spectroscopy (FT-NIR and Micro-NIR) for geographical source areas of coconut milk in tandem with the classical to modern chemometrics classifier. The discrimination model was developed using qualitative chemometrics techniques from classic (Principal Component Analysis-PCA, Partial Least Squares Discriminant Analysis-PLS-DA, Linear Discriminant Analysis-LDA) to modern, including classifiers from machine learning (Support Vector Machine-SVM, k-Nearest Neighbor-KNN, Artificial Neural Network-ANN) and deep learning (Simple Convolutional Neural Networks-S-CNN, S-AlexNET, Residual Networks-ResNET). Three sources as geographical areas of coconut milk originally from Thailand were used, including the south region (Chumphon Province), middle region (Samut Songkhram Province), and east region (Chonburi Province). Our findings showed that a classifier from SVM and ResNET could yield the optimal performance for discriminating the geographical source area of coconut milk using FT-NIR. Furthermore, when using Micro-NIR, the classifier from LDA, SVM, KNN and ResNET delivered the highest accuracy. The performance discrimination models above were excellent when classified based on the kappa coefficient. This study concluded that both FT-NIR and Micro-NIR supported by classical to modern chemometric classifiers could be used to evaluate the geographical area source from coconut milk. Also, the method in this study includes a strategy for discovering feature-important NIR spectra for interpretability purposes, thereby facilitating the qualitative interpretation of results for all types of classifiers.
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Geographical origin identification of Khao Dawk Mali 105 rice using combination of FT-NIR spectroscopy and machine learning algorithms
(2024-10-05)
Lapcharoensuk, Ravipat
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Moul, Chen
The mislabelled Khao Dawk Mali 105 rice coming from other geographical region outside the Thung Kula Rong Hai region is extremely profitable and difficult to detect; to prevent retail fraud (that adversely affects both the food industry and consumers), it is vital to identify geographical origin. Near infrared spectroscopy can be used to detect the specific content of organic moieties in agricultural and food products. The present study implemented the combinatorial method of FT-NIR spectroscopy with chemometrics to identify geographical origin of Khao Dawk Mali 105 rice. Rice samples were collected from 2 different region including the north and northeast of Thailand. NIR spectra data were collected in range of 12,500 – 4,000 cm<sup>−1</sup> (800–2,500 nm). Five machine learning algorithms including linear discriminant analysis (LDA), partial least squares discriminant analysis (PLS-DA), C-support vector classification (C-SVC), backpropagation neural networks (BPNN), hybrid principal component analysis-neural network (PC-NN) and K-nearest neighbors (KNN) were employed to classify NIR data of rice samples with full wavelength and selected wavelength by Extremely Randomized Trees (Extra trees) algorithm. Based on the findings, geographical origin of rice could be specified quickly, cheaply, and reliably using combination of NIRS and machine learning. All models creating by full wavelength and selected wavelength exhibited accuracy between 65 and 100 % for identifying geographical region of rice. It was proven that NIR spectroscopy may be used for the quick and non-destructive identification of geographical origin of Khao Dawk Mali 105 rice.

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