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  4. Mesoscopic Interference of Rotated Spins in Graphene Coupled to High-Spin–Orbit-Coupling Substrates
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Mesoscopic Interference of Rotated Spins in Graphene Coupled to High-Spin–Orbit-Coupling Substrates

Author(s)
Yokoi, Kazushi
Somphonsane, Ratchanok
Ramamoorthy, Harihara
Arabchigavkani, Nargess
He, Keke
Barut, Bilal
Yin, Shenchu
Randle, Michael D.
Dixit, Ripudaman
Nathawat, Jubin
Fransson, Jonas
Kim, Gil Ho
Watanabe, Kenji
Taniguchi, Takashi
Bird, Jonathan P.
Aoki, Nobuyuki
Date Issued
November 5, 2025
Type
Article
DOI
10.1021/acsami.5c15694
Abstract
We explore the manifestations of spin rotation in graphene in proximity with two different types of high-spin–orbit-coupling (SOC) materials (ferromagnetic Co and nominally diamagnetic WSe2). Using weak antilocalization (WAL) as a probe of the induced rotation, we demonstrate that spin interference exhibits a highly stochastic (nonself-averaging) character in the mesoscopic limit. At low temperatures (<20 K), the spin rotation is manifested as a zero-bias peak (or zero-bias anomaly, ZBA) in the differential conductance, a feature that, as expected for WAL, is suppressed by fairly modest magnetic fields (<∼102mT). The ZBA moreover exhibits a stochastic variation when a gate voltage is used to sweep the Fermi level through the graphene bands, with ranges for which the antilocalization is either prominent or strongly suppressed. This mesoscopic character is exhibited by both of the studied systems, whose ZBA is also damped in similar fashion with increasing temperature. We thus provide fundamental insight into the nonensemble-averaged (nonself-averaged) character of spin interference in mesoscopic systems with strong SOC and, more specifically, into how the details of spin rotation are impacted by external gating. This understanding may ultimately enable the efficient modulation of spin currents in future spintronic devices.
Citation
ACS Applied Materials and Interfaces, 17(44), 61050-61058, 2025
Subjects

2D semiconductors

graphene

mesoscopics

spin−orbit coupling

transition-metal dich...

weak antilocalization...

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