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Spin-flop driven magneto-dielectric effect in Co4Nb 2O9

Author(s)
Kolodiazhnyi, T.
Sakurai, H.
Vittayakorn, N.
Date Issued
September 26, 2011
Type
Article
DOI
10.1063/1.3645017
Abstract
Co4Nb2O9 becomes antiferromagnetic (AFM) below 27.4 K with a spin-flop transition at a critical field, Hc, of 12 kOe. Room-temperature dielectric properties are dominated by finite electronic conductivity. Below 125 K, the charge carriers are frozen-out and the dielectric constant is controlled by the lattice phonons. A large (12%) spin flop-driven enhancement in dielectric constant is found in the very narrow temperature interval (ΔT = 1.6 K) in the vicinity of the AFM phase transition. Magneto-dielectric anomaly shows low-frequency dispersion; therefore, the H-induced changes in the phonon eigenfrequencies are unlikely. Other possible reasons for unusual magneto-dielectric effect in Co 4Nb2O9 are discussed. © 2011 American Institute of Physics.
Citation
Applied Physics Letters, 99(13), 2011
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