Effect of the presence of HCl on simultaneous CO2 capture and contaminants removal from simulated biomass gasification producer gas by CaO-Fe2O3 sorbent in calcium looping cycles
| dc.contributor.author | Dashtestani, Forogh | |
| dc.contributor.author | Nusheh, Mohammad | |
| dc.contributor.author | Siriwongrungson, Vilailuck | |
| dc.contributor.author | Hongrapipat, Janjira | |
| dc.contributor.author | Materic, Vlatko | |
| dc.contributor.author | Yip, Alex C.K. | |
| dc.contributor.author | Pang, Shusheng | |
| dc.date.accessioned | 2026-08-06T10:34:02Z | |
| dc.date.available | 2026-08-06T10:34:02Z | |
| dc.date.issued | 2021-12-01 | |
| dc.description.abstract | This study investigated the effect of HCl in biomass gasification producer gas on the CO<inf>2</inf> capture efficiency and contaminants removal efficiency by CaO-Fe<inf>2</inf>O<inf>3</inf> based sorbent material in the calcium looping process. Experiments were conducted in a fixed bed reactor to capture CO<inf>2</inf> from the producer gas with the combined contaminants of HCl at 200 ppmv, H<inf>2</inf>S at 230 ppmv, and NH<inf>3</inf> at 2300 ppmv. The results show that with presence of HCl in the feeding gas, sorbent reactivity for CO<inf>2</inf> capture and contaminants removal was enhanced. The maximum CO<inf>2</inf> capture was achieved at carbonation temperatures of 680<sup>◦</sup>C, with efficiencies of 93%, 92%, and 87%, respectively, for three carbonation-calcination cycles. At this carbonation temperature, the average contaminant removal efficiencies were 92.7% for HCl, 99% for NH<inf>3</inf>, and 94.7% for H<inf>2</inf>S. The outlet contaminant concentrations during the calcination process were also examined which is useful for CO<inf>2</inf> reuse. The pore structure change of the used sorbent material suggests that the HCl in the feeding gas contributes to high CO<inf>2</inf> capture efficiency and contaminants removal simultaneously. | |
| dc.identifier.citation | Energies, 14(23), 2021 | |
| dc.identifier.doi | 10.3390/en14238167 | |
| dc.identifier.issn | 19961073 | |
| dc.identifier.other | 2-s2.0-85120777938 | |
| dc.identifier.uri | https://dspace.kmitl.ac.th/handle/123456789/12415 | |
| dc.source | Energies | |
| dc.subject | Calcium looping | |
| dc.subject | CaO-Fe2O3 sorbent | |
| dc.subject | CO2 capture | |
| dc.subject | Contaminant removal | |
| dc.title | Effect of the presence of HCl on simultaneous CO2 capture and contaminants removal from simulated biomass gasification producer gas by CaO-Fe2O3 sorbent in calcium looping cycles | |
| dc.type | Article |