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High-performance triboelectric and piezoelectric nanogenerator enabled by BF-BT-NZN multifunctional ceramic filler
(2025-10-01)
Sumang, Rattiphorn
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Jantaratana, Pongsakorn
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Charoonsuk, Thitirat
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Vittayakorn, Naratip
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Bongkarn, Theerachai
The development of efficient and flexible energy-harvesting materials is essential for advancing self-powered electronic devices. In this study, we report the fabrication of flexible composite films by incorporating (1-x)(0.75BiFeO<inf>3</inf>-0.25BaTiO<inf>3</inf>)-xNd(Zn<inf>0.67</inf>Nb<inf>0.33</inf>)O<inf>3</inf>,abbreviated as (BF-BT-NZN), ceramic powder into a PDMS matrix, with filler contents ranging from 5 to 25 wt%. The optimized 10 wt% composite film demonstrated a maximum output voltage of 112.24 V and a current of 5.69 µA approximately 11 and 18 times higher than pure PDMS, respectively. Following a poling treatment, the output further increased to 149.54 V and 10.71 µA. The film exhibited excellent flexibility and durability, enabling practical applications such as powering LEDs, a digital watch, and charging capacitors. These results highlight the potential of BF-BT-NZN/PDMS composites as high-performance materials for wearable energy-harvesting applications.
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High-performance flexible lead-free piezo-antiferroelectric based on NaNbO3/PDMS composites for energy harvesting application
(2024-12-01)
Sumang, Rattiphorn
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Charoonsuk, Thitirat
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Vittayakorn, Naratip
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Panpho, Phakakorn
To bring the rapidly advancing technology of energy harvesters into commercial use, further development is required for devices that can enhance output performance, flexibility, ease of fabrication, and low cost. A hybrid concept is a promising method. It combines between the piezoelectric nanogenerator (PENG) and the triboelectric nanogenerator (TENG) to provide a high-performance nanogenerator. This study introduced a high-performance hybrid PENG and TENG device that operates using a NN-BNT/PDMS composite film. The NN-BNT/PDMS composite based nanogenerators were fabricated with varying NN-BNT content. Then, dielectric test and electrical properties were investigated. Adding NN-BNT into the PDMS composite film resulted in a higher dielectric constant compared to pure PDMS, leading to increase of electrical output. Under the optimal condition of a 3 wt%. NN-BNT composite based hybrid nanogenerator, the electrical output was significantly enhanced, reaching 40 V, 0.95 μA/cm<sup>2</sup>, and 200 μW/cm<sup>2</sup> compared to pure PDMS. This nanogenerator further used to the charging of a capacitor to a voltage of around 1 V within 5 s and also powered multiple LEDs. The successful development of this highly efficient NN-BNT/PDMS composite film-based hybrid concept sheds light on energy harvesting devices.
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Influence of pore morphologies on the mechanical and tribo-electrical performance of polydimethylsiloxane sponge fabricated via commercial seasoning templates
(2021-12-01)
Pharino, Utchawadee
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Sinsanong, Yoltawan
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Pongampai, Satana
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Charoonsuk, Thitirat
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Pakawanit, Phakkhananan
This work demonstrated the influence of pore morphologies on the mechanical behavior and tribo-electrical performance of fabricated polydimethylsiloxane (PDMS) sponge. Commercial seasonings with different 3D geometric shapes were used as a sacrificial template to control the pore structure of the PDMS sponge. The result indicated that the softest PDMS sponge was molded by using a sodium chloride (NaCl) crystal template, as indicated by the lowest compressive modulus value. Then, P(VDF–HFP) was incorporated into PDMS prepolymer in order to enhance the charge generation characteristic of PDMS. Besides, the composite 3D structure was revealed using synchrotron radiation X-ray tomographic microscopy (SRXTM). Interpretation from the SRXTM result confirmed that the porous structure had different pore shapes, i.e., an octahedral-like shape and a circular-like shape in a particular sponge. By pairing the composite PDMS sponge with an aluminum (Al) plate for the triboelectric nanogenerator (TENG), the maximum electrical outputs of ~29.9 V and ~0.56 μA for voltage and current, respectively, were detected with loading 50 wt% of P(VDF – HFP). The presented TENG was applied successfully for sensing basic human activities practically, which demonstrated potential applications in wearable electronics.
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High Performance Flexible Tribo/Piezoelectric Nanogenerators based on BaTiO3/Chitosan Composites
(2021-01-01)
Pongampai, Satana
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Charoonsuk, Thitirat
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Pinpru, Nattapong
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Muanghlua, Rangson
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Vittayakorn, Wanwilai
Natural biopolymer materials have been of interest in wearable energy harvester technology, especially in biocompatible triboelectric nanogenerators (BTENGs), due to their biodegradable, biocompatible, nontoxic and excellent antibacterial properties. Nevertheless, obstacles concerning economical and biocompatible utilization of triboelectric nanogenerators (TENGs) continue to prevail. The natural biopolymer, chitosan (CS), is composed of a long biopolymer chain of N-acetyl glucosamine. It enables exciting opportunities for low-cost, biodegradable triboelectric nanogenerator (TENG) applications. However, the electrical output performance of CS based on TENGs is low when compared with devices constructed from synthetic polymers. Hence, to enhance electrical output performance, BaTiO<inf>3</inf> nano-powders (BT-NPs) were embedded into the CS as dielectric material, in order to improve electrical properties by increasing the dielectric constant of the composite film. A flexible hybrid piezo/triboelectric nanogenerator, designed by BT-NPs embedded into CS (BT-NPs/CS) composite film, was constructed successfully. The effects of the BaTiO<inf>3</inf> nano-powder (BT-NP) content on the output performance were explored systematically. The device with 5 wt% BT-NPs in CS, and a 160-μm-thick film, exhibited maximum open-circuit voltage (V<inf>OC</inf>) and transferred short-circuit current (I<inf>SC</inf>) of 110.8 V and 10 µA, respectively, as well as maximum power output of 431.8 µW. Practical and application demonstrations also were investigated, namely charged capacitors for storing energy, testing voltage stability and driving commercial LEDs. This work exhibited high electrical performance enhancement of BT-NPs/CS nanocomposite film, which demonstrated better material modification.
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Effect of surface treatment on electrical properties of polydimethylsiloxane based triboelectric nanogenerator
(2020-01-01)
Panprom, Parinya
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Vittayakorn, Naratip
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Nawanil, Chanisa
This research investigated the effect of surface treatment on electrical properties of flexible triboelectric nanogenerator (TENG). Polydimethylsiloxane (PDMS) was used as triboelectric layer. The PDMS pads were prepared by simple casting method and the effect of surface treatments by heat and acid was examined. Physical morphology of treated samples were investigated by scanning electron microscope (SEM). Electrical properties were measured under continuous periodic knocking. The results revealed that the heat-treated PDMS-based TENG showed the outstanding output voltage. The maximum output voltage of heat-treated based TENG reached approximately 9 V, which was over 4 times larger than those of normal PDMS based TENG. The research demonstrated the feasibility to utilize PDMS-based TENG as an energy harvesting device and presented a cost-effective method for producing high-efficiency PDMS based TENG.

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